+1 for Tube Saturation found in the Pro Channel. This will give you a distorted vocal, something akin to The Beatles I Am The Walrus.
Another option is using an amp sim, again to create distortion along with a pitch shifter. I particularly like Guitar Rig 4s octave pedal or Waves Doubler for this effect.
Finally, the old fashioned way is to sing yourself hoarse...like Jim Morrison, just scream into a SM58 or something like that and you should get a gravelly effect.
I don't recommend you take up smoking like Freddie Mercury did, he smoked or so the story goes because he liked the gravelly effect it gave his voice in later years...I'm not sure how many smokes a day and how long it took to get that effect...it also gave him throat nodules too.
:)