In my experience, crackles and pops have always had more to do with the audio drivers and the interface they are connected to. For a firewire interface card/chipset, a Texas Instruments based chipset is what I've had the best results with.
I very much doubt that an SSD drive would cure your problems. I will say though, that another hard drive added to your system would be beneficial. I currently have an SSD drive for OS and programs, a dedicated drive for samples and a dedicated drive for multi-track audio recording.
You can get a 1TB hard drive for around $50. Install it and use it for your multi-track recordings and see what happens. If it doesn't work out, you can always use it as a back-up drive. Of course, if you have money to burn, go ahead and get an SSD.