Really depends on your thrust, musically
I am not that enamored with the mega magic series, although they're wonderful, compared to most things on the market. But considering all things Guru, I tend to gravitate much more to Airwave 1 and 2, which are just f'n blowminds, Galactic, Northern Lights, Sabersphere 1/2, Kid 2, and OMG are all very lovely. Almost ALL the guru's libraries are superior as they add sample content and some serious juju on effects and controllers. The polifany of contributors to each recent library also ups the quality as each contributor is stellar in their own right.
Will have to check out
Realm... The naked demos I'm listening to sound awesome!
Collossus is ok. Tiring of Matt though... pretty simple stuff and no deep innovations. This maybe a bit harsh as among the zillion patches there are lots of nice things.
Luftdrum and Hollo are pretty amazing, given that they do it all with existing samples. They put out just a few but extremely well crafted libraries.